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With [MN2 )(P2Me PP2Ph )] the initial Chatt-type complex with one coordination site catalytically converting N2 to ammonia is presented. Employing SmI2 as reductant and H2 O as proton source 26 equivalents of ammonia are produced. Analogous Mo0 -N2 complexes supported by a mixture of bi- and tridentate phosphine ligands tend to be catalytically inactive under the same problems. These findings tend to be translated by examining architectural and spectroscopic features of the utilized methods, causi
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