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A very minor ground-state C5H8 + CH3 channel is observed, attributed predominantly to 1,3-pentadiene formation. The ground-state branching ratios agree well with RRKM calculations, which also predict C4H6 + C2H5 and C3H6 + C3H5 channels with similar yield to C5H8 + CH3. If these channels were active, it was at levels too low to be observed.We present a systematic approach for the identification of statistically relevant conformational macrostates of organic molecules from molecular dynamics trajectories. The approach applies to molecules

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