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Bayer red mud (RM) occupies a large amount of land, which excessive Na+ seriously damages groundwater resources. In this research, a RM based cementitious material (RMC) composed of RM and ordinary Portland cement (OPC) was developed. It is interesting to find that a binary reaction consisting of cement hydration and geopolymer reaction in RMC. The mechanical and Na+ consolidation rate of RMC were improved by the synergistic effect of binary reaction. The results indicated that the compressive strength of RMC is the highest and reaches 32.