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The contributions of spin-phonon coupling (SPC) to spin and thermal transport properties are important in emerging two-dimensional (2D) magnetic semiconductors and are relevant to the data security and working stability of spin-based devices. By evaluating the dynamical stability of both ferromagnetic (FM) and paramagnetic (PM) states at 0 K, six transition-metal trihalides, namely FeCl3, FeBr3, FeI3, RuCl3, RuBr3, and RuI3, are identified as ideal 2D magnetic semiconductors for investigating SPC. For these compounds, we perform first-pr

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