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This back reduction was further verified to be exergonic via reactive Gibbs free energy, indicating the back reduction by humic substances of CTC oxidation intermediates could occur spontaneously. The present study will be helpful for predicting the fate and risk of CTC in algae rich water environments, and is of great significance for the study of phototransformation of other antibiotics.It is known that sludge dewaterability improves during the thermal hydrolysis process (THP); however, the effect of thermal hydrolysis and