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Hybrid heterojunction solar cells (HHSCs) using crystalline Si nanowires (SiNWs) as the absorber and conducting polymer poly(3,4-ethylenedioxythiophene)poly(styrenesulfonate) (PEDOTPSS) as the hole-selective transport layer (HTL) show great potential in both low-cost and high-power conversion efficiency (PCE). However, due to the poor wettability of the PEDOTPSS solution on SiNWs, conformal coverage of PEDOTPSS on SiNWs is not easy to achieve. Here, an effective method was developed to decrease the surface tension of the PEDOTPSS and inc