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This is an important outcome indicating that nanoplastic stability and dispersion state will be more pronounced and therefore more challenging to eliminate. Results highlight the key role of NP and PS nanoplastic surface charge, as well as water properties, coagulant type, and dosage on nanoparticle elimination from aquatic systems. PRACTITIONER POINTS pH, water hardness, and NOM are playing roles in final coagulant dosage concentration. PACl is more efficient than FeCl3 in most conditions. Positively charged nanoplastics are more